Forum for Science, Industry and Business

Sponsored by:     3M 
Search our Site:

 

Sharper nanoscopy

20.03.2015

What happens when a quantum dot looks in a mirror?

The 2014 chemistry Nobel Prize recognized important microscopy research that enabled greatly improved spatial resolution. This innovation, resulting in nanometer resolution, was made possible by making the source (the emitter) of the illumination quite small and by moving it quite close to the object being imaged.


This is an illustration of the interference between light from the quantum dot (black sphere) and radiation from the mirror dipole (black sphere on the wire). This interference will slightly distort the perceived location of the diffraction spot as imaged on a black screen at the top. The distortion is different depending on whether the quantum dot dipole is oriented perpendicular (red) or parallel (blue) to the wire surface, a difference that can be visualized by imaging the diffraction spot along different polarizations.

Credit: Ropp

One problem with this approach is that in such proximity, the emitter and object can interact with each other, blurring the resulting image. Now, a new JQI study has shown how to sharpen nanoscale microscopy (nanoscopy) even more by better locating the exact position of the light source.

Diffraction limit

Traditional microscopy is limited by the diffraction of light around objects. That is, when a light wave from the source strikes the object, the wave will scatter somewhat. This scattering limits the spatial resolution of a conventional microscope to no better than about one-half the wavelength of the light being used. For visible light, diffraction limits the resolution to no be better than a few hundred nanometers.

How then, can microscopy using visible light attain a resolution down to several nanometers? By using tiny light sources that are no larger than a few nanometers in diameter. Examples of these types of light sources are fluorescent molecules, nanoparticles, and quantum dots. The JQI work uses quantum dots which are tiny crystals of a semiconductor material that can emit single photons of light. If such tiny light sources are close enough to the object meant to be mapped or imaged, nanometer-scale features can be resolved. This type of microscopy, called "Super-resolution imaging," surmounts the standard diffraction limit.

Image-dipole distortions

JQI fellow Edo Waks and his colleagues have performed nanoscopic mappings of the electromagnetic field profile around silver nano-wires by positioning quantum dots (the emitter) nearby. (Previous work summarized at http://jqi.umd.edu/news/using-single-quantum-dots-probe-nanowires).

They discovered that sub-wavelength imaging suffered from a fundamental problem, namely that an "image dipole" induced in the surface of the nanowire was distorting knowledge of the quantum dot's true position. This uncertainty in the position of the quantum dot translates directly into a distortion of the electromagnetic field measurement of the object.

The distortion results from the fact that an electric charge positioned near a metallic surface will produce just such an electric field as if a ghostly negative charge were located as far beneath the surface as the original charge is above it. This is analogous to the image you see when looking at yourself in a mirror; the mirror object appears to be as far behind the mirror as you are in front. The quantum dot does not have a net electrical charge but it does have a net electrical dipole, a slight displacement of positive and negative charge within the dot.

Thus when the dot approaches the wire, the wire develops an "image" electrical dipole whose emission can interfere with the dot's own emission. Since the measured light from the dot is the substance of the imaging process, the presence of light coming from the "image dipole" can interfere with light coming directly from the dot. This distorts the perceived position of the dot by an amount which is 10 times higher than the expected spatial accuracy of the imaging technique (as if the nanowire were acting as a sort of funhouse mirror).

The JQI experiment successfully measured the image-dipole effect and properly showed that it can be corrected under appropriate circumstances. The resulting work provides a more accurate map of the electromagnetic fields surrounding the nanowire.

The JQI scientists published their results in the journal Nature Communications.

Lead author Chad Ropp (now a postdoctoral fellow at the University of California, Berkeley) says that the main goal of the experiment was to produce better super-resolution imaging: "Any time you use a nanoscale emitter to perform super-resolution imaging near a metal or high-dielectric structure image-dipole effects can cause errors. Because these effects can distort the measurement of the nano-emitter's position they are important to consider for any type of super-resolved imaging that performs spatial mapping."

"Historically scientists have assumed negligible errors in the accuracy of super-resolved imaging," says Ropp. "What we are showing here is that there are indeed substantial inaccuracies and we describe a procedure on how to correct for them."

###

Reference report: "Nanoscale probing of image dipole interactions in a metallic nanostructure," Chad Ropp, Zachary Cummins, Sanghee Nah, John T. Fourkas, Benjamin Shapiro, Edo Waks, Nature Communications, 19 March 2015; Doi:10.1038/ncomms7558 http://www.nature.com/ncomms/2015/150319/ncomms7558/full/ncomms7558.html

Media Contact

Phillip F. Schewe
pschewe@umd.edu
301-405-0989

http://jqi.umd.edu 

Phillip F. Schewe | EurekAlert!
Further information:
http://www.jqi.umd.edu

More articles from Physics and Astronomy:

nachricht Breakthrough with a chain of gold atoms
17.02.2017 | Universität Konstanz

nachricht New functional principle to generate the „third harmonic“
16.02.2017 | Laser Zentrum Hannover e.V.

All articles from Physics and Astronomy >>>

The most recent press releases about innovation >>>

Die letzten 5 Focus-News des innovations-reports im Überblick:

Im Focus: Breakthrough with a chain of gold atoms

In the field of nanoscience, an international team of physicists with participants from Konstanz has achieved a breakthrough in understanding heat transport

In the field of nanoscience, an international team of physicists with participants from Konstanz has achieved a breakthrough in understanding heat transport

Im Focus: DNA repair: a new letter in the cell alphabet

Results reveal how discoveries may be hidden in scientific “blind spots”

Cells need to repair damaged DNA in our genes to prevent the development of cancer and other diseases. Our cells therefore activate and send “repair-proteins”...

Im Focus: Dresdner scientists print tomorrow’s world

The Fraunhofer IWS Dresden and Technische Universität Dresden inaugurated their jointly operated Center for Additive Manufacturing Dresden (AMCD) with a festive ceremony on February 7, 2017. Scientists from various disciplines perform research on materials, additive manufacturing processes and innovative technologies, which build up components in a layer by layer process. This technology opens up new horizons for component design and combinations of functions. For example during fabrication, electrical conductors and sensors are already able to be additively manufactured into components. They provide information about stress conditions of a product during operation.

The 3D-printing technology, or additive manufacturing as it is often called, has long made the step out of scientific research laboratories into industrial...

Im Focus: Mimicking nature's cellular architectures via 3-D printing

Research offers new level of control over the structure of 3-D printed materials

Nature does amazing things with limited design materials. Grass, for example, can support its own weight, resist strong wind loads, and recover after being...

Im Focus: Three Magnetic States for Each Hole

Nanometer-scale magnetic perforated grids could create new possibilities for computing. Together with international colleagues, scientists from the Helmholtz Zentrum Dresden-Rossendorf (HZDR) have shown how a cobalt grid can be reliably programmed at room temperature. In addition they discovered that for every hole ("antidot") three magnetic states can be configured. The results have been published in the journal "Scientific Reports".

Physicist Dr. Rantej Bali from the HZDR, together with scientists from Singapore and Australia, designed a special grid structure in a thin layer of cobalt in...

All Focus news of the innovation-report >>>

Anzeige

Anzeige

Event News

Booth and panel discussion – The Lindau Nobel Laureate Meetings at the AAAS 2017 Annual Meeting

13.02.2017 | Event News

Complex Loading versus Hidden Reserves

10.02.2017 | Event News

International Conference on Crystal Growth in Freiburg

09.02.2017 | Event News

 
Latest News

Switched-on DNA

20.02.2017 | Materials Sciences

Second cause of hidden hearing loss identified

20.02.2017 | Health and Medicine

Prospect for more effective treatment of nerve pain

20.02.2017 | Health and Medicine

VideoLinks
B2B-VideoLinks
More VideoLinks >>>