In the experiments, an electron in a krypton atom is removed by a laser pulse that lasts less than four femtoseconds (one femtosecond is one millionth of one billionth of a second). This process leaves behind an atom with a pulsating positively charged hole in the valence shell, which originates from electronic wave functions of the atom.
The scientists led by Dr. Steve Leone, an ultrafast laser expert and the recent recipient of a National Security Science and Engineering Faculty Fellowship, used an extreme ultraviolet light pulse, the duration for which was 150 attoseconds (one attosecond is one billionth of one billionth of a second), to capture and photograph the movement of valence electrons for the first time.
This research into electron motions is expected to enable the scientists to better control processes and materials that will improve high-speed electronics and carbon-free energy sources that will benefit both the Air Force and consumers.
"If we want to understand high speed electronics, we need to work on changing molecular bonds in chemical reactions and the movement of electrons during chemical reactions or in complex solids which will only be possible by freezing time in a femtosecond," said Leone.
Dr. Michael R. Berman, program manager at AFOSR who is overseeing the scientists believes their research is an elegant example of the new capabilities of attosecond pulses to probe the dynamics of electron motions.
"This program and instrumentation will open new doors into probing fundamental physical processes on time scales faster than ever probed before."
Berman also noted, "These new tools will let us probe electron dynamics in materials and semiconductors and could help us understand and reduce electron loss processes to make electronics and devices like solar cells more efficient and to bring electronic data processing to its highest level."ABOUT AFOSR:
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A newly developed laser technology has enabled physicists in the Laboratory for Attosecond Physics (jointly run by LMU Munich and the Max Planck Institute of Quantum Optics) to generate attosecond bursts of high-energy photons of unprecedented intensity. This has made it possible to observe the interaction of multiple photons in a single such pulse with electrons in the inner orbital shell of an atom.
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A group of researchers led by Andrea Cavalleri at the Max Planck Institute for Structure and Dynamics of Matter (MPSD) in Hamburg has demonstrated a new method enabling precise measurements of the interatomic forces that hold crystalline solids together. The paper Probing the Interatomic Potential of Solids by Strong-Field Nonlinear Phononics, published online in Nature, explains how a terahertz-frequency laser pulse can drive very large deformations of the crystal.
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For the first time, a team of researchers at the Max-Planck Institute (MPI) for Polymer Research in Mainz, Germany, has succeeded in making an integrated circuit (IC) from just a monolayer of a semiconducting polymer via a bottom-up, self-assembly approach.
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